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Citation - WoS: 6
Citation - Scopus: 5
Structural and Optical Characteristics of Antimony Selenosulfide Thin Films Prepared by Two-Step Method
(Springer, 2022) Türkoğlu, Fulya; Ekren, Memduh Emirhan; Cantaş, Ayten; Yakıncı, Kübra; Gündoğan, Hazal; Aygün, Gülnur; Özyüzer, Lütfi
Antimony triselenide (Sb2Se3) is one of the most promising absorber material choices among the inorganic semiconductors that has attracted much attention today. However, highest recorded efficiencies for Sb2Se3 solar cells are still lower than ideal. Exploring antimony selenosulfide (Sb-2(SxSe1-x)(3)) to increase device performance is one option because some features of alloyed Sb-2(SxSe1-x)(3) depend on composition such as bandgap and band position. In this study, two-step process was used to grow Sb-2(SxSe1-x)(3) thin films. In the first stage, Sb2Se3 thin films were deposited on soda lime glass substrates using direct current magnetron sputtering technique. In the second stage, Sb2Se3 thin films were exposed to sulfurization process in a quartz ampoule to obtain Sb-2(SxSe1-x)(3) thin films. Characterization results showed that morphological, optical, and structural properties of Sb-2(SxSe1-x)(3) thin films grown by presented method were highly dependent on amount of sulfur in the films. By the adjustment of the S/S + Se atomic ratio, Sb-2(SxSe1-x)(3) absorber materials with suitable bandgap, favorable orientation and compact morphology can be obtained for photovoltaic applications.
Citation - WoS: 2
Citation - Scopus: 2
Enhancing the Photo-Response Characteristics of Graphene/N-si Based Schottky Barrier Photodiodes by Increasing the Number of Graphene Layers
(AVS, 2022) Fidan, Mehmet; Ünverdi, Özhan; Çelebi, Cem
The impact of the number of graphene layers on the spectral responsivity and response speed of graphene/n-type Si (Gr/n-Si)-based Schottky barrier photodiodes is investigated. Gr/n-Si photodiode devices are fabricated by transferring chemical vapor deposition-grown graphene layers one by one on n-Si substrates, reaching up to three graphene layers. The devices show a clear rectifying Schottky character and have a maximum responsivity at a peak wavelength of 905 nm. Wavelength-resolved and time-dependent photocurrent measurements demonstrated that both spectral responsivity and response speed are enhanced as the number of graphene layers is increased from 1 to 3 on n-Si substrates. For example, the spectral responsivity and the response speed of the fabricated device were found to be improved by about 15% (e.g., from 0.65 to 0.75 AW-1) and 50% (e.g., 14 to 7 μs), respectively, when three graphene layers are used as the hole-collecting cathode electrode. The experimentally obtained results showed that the device parameters, such as spectral responsivity and response speed of Gr/n-Si Schottky barrier photodiodes, can be boosted simply by increasing the number of graphene layers on n-Si substrates.
Citation - WoS: 3
Citation - Scopus: 3
Atomic-Scale Investigation of the Effect of Surface Carbon Coatings on the Oxidation and Mechanical Properties of Iron Nanowires
(Royal Society of Chemistry, 2021) Aral, Gürcan; Islam, Md Mahbubul
The understanding of the complex atomistic-scale mechanisms of the oxidation process of carbon (C) coated iron nanowires (Fe NW) and also the resulting modulation of mechanical properties is a highly challenging task. We perform reactive molecular dynamics (RMD) simulations based on the ReaxFF force field to investigate the mechanisms of the oxidation process of [001]-oriented pristine cylindrical Fe NWs with and without a C coating in an O2 environment in order to obtain detailed insights into the influences of the surface C coating on the oxidation process at room temperature. Here, we show that the C-coated shell layer on the free surface of pristine Fe NWs partially controls the spontaneous oxidation when exposed to O2 molecules by hindering the absorption-dissociation of O2 molecules and diffusion of O ions into the shell layer. In particular, the surface modification of the pristine Fe NW with the C-coated shell layer has pronounced effects on the improvement of oxidation resistance by lowering the surface reactivity, which limits the formation of an oxide shell layer on the free surface of the NW. The formation of strong Fe-C bonds in the C-coated shell layer largely restrains the oxidation process. Furthermore, to examine the influence of the C-coated shell layer on the resulting modulation of mechanical properties of the pristine Fe NW, we systematically investigate the mechanical deformation processes and related properties of Fe NW with and without a C coating including their oxidized counterparts subjected to both uniaxial tensile and compressive loads at room temperature. The yield stress and strain (the elastic limit) of Fe NWs including the elastic and plastic deformation phase of the stress-strain relationship are found to be sensitive to the loading modes, the existence of the C-coated shell layer and the resulting formation of an oxide shell layer on the surface of the C-coated Fe NW.

Physics / Fizik

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