Physics / Fizik
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Conference Object Probing the Density of States of High Temperature Superconductors With Point Contact Tunneling Spectroscopy(Springer Verlag, 2005) Özyüzer, Lütfi; Zasadzinski, John F.; Miyakawa, Nobuaki; Gray, Kenneth E.Tunneling spectroscopy measurements are performed on single crystals of single CuO2 layer Tl2Ba2CuO6+delta, double CuO2 layer Bi2Sr2CaCu2O8+delta (Bi2212) and polycrystal quadruple CuO2 layer CuBa2Ca3Cu4O12+delta using the point contact tunneling technique. I-V and dI/dV-V characteristics are obtained at 4.2 K. In spite of different number of layers and T-c values, all three high-T-c superconductors exhibit similar spectral features including dip and hump features reminiscent of strong-coupling effects in conventional superconductors. The doping dependence of Bi2212 is studied and several effects of the hole concentration on spectral features are found. A novel effect is that the energy gap increases in the underdoped region even as T-c decreases. Combining the doping dependence of the energy gap and the dip energy provides additional information in order to understand the mechanism of high-T-c superconductivity. Point contact tunneling studies of the doping dependence of the energy gap in Bi2212 also helped to understand local variations of the gap magnitude observed by scanning tunneling microscopy, indicating that this type of spectroscopy is an integral part of the tunneling technique.Article Citation - WoS: 150Citation - Scopus: 7Correlation of Tunneling Spectra in Bi2sr2cacu2o8+? With the Resonance Spin Excitation(American Physical Society, 2001) Zasadzinski, John F.; Özyüzer, Lütfi; Miyakawa, Nobuaki; Gray, Kenneth E.; Hinks, David G.; Kendziora, Christopher A.New break-junction tunneling data are reported in Bi2Sr2CaCu2O8+δ over a wide range of hole concentration from underdoped (Tc=74k) to optimal doped (Tc=95k) to overdoped (Tc=48k). The conductances exhibit sharp dips at a voltage, Ω/e, measured with respect to the superconducting gap. Clear trends are found such that the dip strength is maximum at optimal doping and that Ω scales as 4.9kTc over the entire doping range. These features link the dip to the resonance spin excitation and suggest quasiparticle interactions with this mode are important for superconductivity.Article Citation - WoS: 16Citation - Scopus: 18Tunneling Studies of Multilayered Superconducting Cuprate (cu,c)ba2ca3cu4o12+?(World Scientific Publishing Co. Pte Ltd, 2003) Miyakawa, Nobuaki; Tokiwa, K.; Mikusu, S.; Zasadzinski, John F.; Özyüzer, Lütfi; İshihara, T.; Kaneko, Tsutomu; Watanabe, T.; Gray, Kenneth E.Point contact tunneling data are reported in a multilayered high-T c cuprate (Cu,C)Ba2Ca3Cu4O 12+δ with Tc = 117 K. The tunneling spectra in the superconducting state (T ≪ Tc) display spectral features such as well-defined superconducting gap peak at ±Δ as well as dip-hump structures beyond the peaks. In some cases, the spectra with two-gaps have been observed, indicating the coexistence of two inequivalent superconducting layers. The statistical distribution of superconducting gap magnitude suggests two distinct kinds of superconducting gaps that may originate from two inequivalent CuO2 planes, a characteristics of multilayered cuprates with n ≥ 3.Article Citation - WoS: 2Citation - Scopus: 3Reply To "comment on 'counterintuitive Consequence of Heating in Strongly-Driven Intrinsic Junctions of Bi2sr2cacu 2o8+? Mesas'"(American Physical Society, 2011) Kurter, Cihan; Özyüzer, Lütfi; Proslier, Thomas; Zasadzinski, John F.; Hinks, David G.; Gray, Kenneth E.The main criticism raised in the preceding Comment concerns our suggestion that sharp conduction peaks in Bi 2Sr 2CaCu 2O 8+δ mesas, along with absent dip-hump features, may, in general, be a result of self-heating. The author points to the variety of experimental configurations, matrix-element effects, and doping dependencies that might allow a diversity of conductance spectra. We argue that numerous mesa studies (with fixed matrix elements) firmly establish the systematic development of sharp conductance peaks with increased self-heating, and thus, the issue of nonuniversality of tunneling characteristics is not relevant. The author mentions a number of studies that show that the mesa is superconducting near the conductance peak voltage. This is not in dispute and indicates a misinterpretation of our analysis that is clarified here. To address further comments on the technical details of our heating model, we reiterate that our conclusions are independent of our model but rather are based solely on experimental data that are not in dispute.Article Citation - WoS: 2Citation - Scopus: 2The Icrn Value in Intrinsic Josephson Tunnel Junctions in Bi2sr2cacu2o8+? (bi2212) Mesas(Springer Verlag, 2011) Kurter, Cihan; Özyüzer, Lütfi; Hinks, David G.; Gray, Kenneth E.; Zasadzinski, John F.The c-axis current-voltage I(V) characteristics have been obtained on a set of mesas of varying height sculpted on Bi2Sr2CaCu2O8+δ (Bi2212) crystals intercalated with HgB2. The intercalation, along with the small number of junctions in the mesa, N = 6–30, minimizes the degree of self-heating, leading to a consistent Josephson critical current, IC, among junctions in the mesa. The Bi2212 crystals with a bulk TC =74 K are overdoped and display negligible pseudogap effects allowing an accurate measure of the normal state resistance, RN. These properties make themesas nearlyideal for the determinationof the Josephson ICRN product.Wefind ICRN valuesconsistently ∼30% of the quasiparticle gap parameter, /e, which was measured independently using a mechanical contact, break junction technique. The latter was necessitated by higher bias heating effects in the mesas which prevented direct measurements of the superconducting gap. These values are among the highest reported and may represent the maximum intrinsic value for ICRN. The results indicate that the c-axis transport is a mixture of coherent and incoherent tunneling.Article Citation - WoS: 42Citation - Scopus: 43Counterintuitive Consequence of Heating in Strongly-Driven Intrinsic Junctions of Bi2 Sr2 Cacu2 O 8+? Mesas(American Physical Society, 2010) Kurter, Cihan; Özyüzer, Lütfi; Proslier, T.; Zasadzinski, John F.; Hinks, David G.; Gray, Kenneth E.Anomalously high and sharp peaks in the conductance of intrinsic Josephson junctions in Bi2 Sr2 CaCu2 O 8+δ (Bi2212) mesas have been commonly interpreted as superconducting energy gaps but here we show they are a result of strong self-heating. This conclusion follows directly from a comparison to the equilibrium gap measured by tunneling in single break junctions on equivalent crystals. As the number of junctions in the mesa, N, and thus heating increase, the peak voltages decrease and the peak width abruptly sharpens for N≥12. Clearly these widely variable features vs N cannot all represent the equilibrium properties. Our data imply that the sharp peaks represent a transition to the normal state. That it occurs at the same dissipated power for N=12-30 strongly implicates heating as the cause. Although peak sharpening due to heating is counterintuitive, as tunneling spectra usually broaden at higher temperatures, a lateral temperature gradient, leading to coexistence of normal hot spots and superconductive regions, qualitatively explains the behavior. However, a more uniform temperature profile cannot be ruled out. As the peak's width and voltage in our shortest mesa (N=6) are more consistent with the break junction data, we propose a figure of merit for Bi2212 mesas, the relative conductance peak width, such that small values signal a crossover into the strong self-heating regime. © 2010 The American Physical Society.Conference Object Citation - WoS: 36Citation - Scopus: 40Thermal Management in Large Bi2212 Mesas Used for Terahertz Sources(Institute of Electrical and Electronics Engineers Inc., 2009) Kurter, Cihan; Gray, Kenneth E.; Zasadzinski, John F.; Özyüzer, Lütfi; Koshelev, A. E.; Li, Q.; Yamamoto, T.; Kadowaki, K.; Kwok, W. K.; Tachiki, M.; Welp, U.We present a thermal analysis of a patterned mesa on a Bi 2Sr2CaCu2O8 (Bi2212) single crystal that is based on tunneling characteristics of the c-axis stack of ∼800 intrinsic Josephson junctions in the mesa. Despite the large mesa volume (e.g., 40 × 300 × 1.2 μm3) and power dissipation that result in self-heating and backbending of the current-voltage curve (I-V), there are accessible bias conditions for which significant polarized THz-wave emission can be observed. We estimate the mesa temperature by equating the quasiparticle resistance, Rqp(T), to the ratio V/I over the entire I-V including the backbending region. These temperatures are used to predict the unpolarized black-body radiation reaching our bolometer and there is substantial agreement over the entire I-V. As such, backbending results from the particular R qp (T) for Bi2212, as first discussed by Fenton, rather than a significant suppression of the energy gap. This model also correctly predicts the observed disappearance of backbending above ∼60 K.Article Citation - WoS: 150Citation - Scopus: 146Direct Observation of Tetrahertz Electromagnetic Waves Emitted From Intrinsic Josephson Junctions in Single Crystalline Bi2sr2cacu2o8+?(Elsevier Ltd., 2008) Kadowaki, K.; Yamaguchi, H.; Kawamata, K.; Yamamoto, T.; Minami, H.; Kakeya, I.; Welp, U.; Özyüzer, Lütfi; Koshelev, A. E.; Kurter, Cihan; Gray, Kenneth E.; Kwok, W. K.We have observed intense, coherent, continuous and monochromatic electromagnetic (EM) emission at terahertz frequencies generated from a single crystalline mesa structure of the high-Tc superconductor Bi2Sr2CaCu2O8+δ intrinsic Josephson junction system. The mesa is fabricated by the Argon-ion-milling and photolithography techniques on the cleaved surface of Bi2Sr2CaCu2O8+δ single crystal. The frequency, ν, of the EM radiation observed from the sample obeys simple relations: ν = c/nλ = c/2nw and ν = 2eV/hN, where c is the light velocity in vacuum, n the refractive index of a superconductor, λ the wave length of the EM emission in vacuum, w the shorter width of the mesa, V the voltage applied to the mesa, N the number of layers of intrinsic Josephson junctions, e and h are the elementary charge and the Planck constant, respectively. These two relations strongly imply that the mechanism of the emission is, firstly, due to the geometrical resonance of EM waves to the mesa like a cavity resonance occuring in the mesa structure, and forming standing waves as cavity resonance modes, and secondly, due to the ac-Josephson effect, which works coherently in all intrinsic Josephson junctions. The peculiar temperature dependence of the power intensity emitted form samples shows a broad maximum in a temperature region between 20 and 40 K, suggesting that the nonequilibrium effect plays an essential role for the emission of EM waves in this system. The estimated total power is significantly improved in comparison with the previous report [L. Ozyuzer et al., Science 318 (2007) 1291, K. Kadowaki, et al., Physica C 437-438 (2006) 111, I.E. Batov, et al., Appl. Phys. Lett. 88 (2006) 262504], and reached as high as 5 μW from single mesa with w = 60 μm at 648 GHz, which enables us to use it for some of applications. So far, we succeeded in fabricating the mesa emitting EM waves up to 960 GHz in the fundamental mode in the w = 40 μm mesa, whereas the higher harmonics up to the 4-th order were observed, resulting in a frequency exceeding 2.5 THz. In sharp contrast to the previous reports [K. Kadowaki, et al., Physica C 437-438 (2006) 111, M.-H. Bae, et al., Phys. Rev. Lett. 98, (2007) 027002], all the present measurements were done in zero magnetic field. Lastly, a plausible theoretical model for the mechanism of emission is discussed.Article Citation - WoS: 40Citation - Scopus: 45Terahertz Wave Emission From Intrinsic Josephson Junctions in High- Tc Superconductors(IOP Publishing Ltd., 2009) Özyüzer, Lütfi; Şimşek, Yılmaz; Köseoğlu, Hasan; Türkoğlu, Fulya; Kurter, Cihan; Welp, U.; Koshelev, A. E.; Gray, Kenneth E.; Kwok, W. K.; Yamamoto, T.; Kadowaki, K.; Koval, Yu I.; Wang, Huabing; Müller, Paul H.Recently, we experimentally demonstrated that rectangular mesa structures of intrinsic Josephson junctions (IJJ) in Bi2Sr2CaCu 2O8+d (Bi2212) can be used as a compact solid-state generator of continuous, coherent and polarized terahertz (THz) radiation. In the present work, we will exhibit tall mesas (over 600 junctions) which were fabricated using UV lithography, e-beam lithography with photoresist and e-beam lithography with a Ti selective etching technique. We will present measurements of the c-axis resistance as a function of temperature and of current-voltage characteristics of THz emitting mesas with lateral sizes ranging from 30 × 300 to 100 × 300νm2. Furthermore, we will discuss the dependence of the characteristics of the mesa structures on the oxygen doping level of the Bi2212 crystals. We will also experimentally show that the voltage-frequency relation of the ac Josephson effect has to match the cavity resonance for successful emission.Article Citation - WoS: 54Citation - Scopus: 55Persistence of Strong Electron Coupling To a Narrow Boson Spectrum in Overdoped Bi2sr2cacu2o8+î Tunneling Data(American Physical Society, 2006) Zasadzinski, John F.; Özyüzer, Lütfi; Coffey, L.; Gray, Kenneth E.; Hinks, David G.; Kendziora, Christopher A.A d-wave, Eliashberg analysis of break-junction and STM tunneling spectra on Bi2Sr2CaCu2O8+Î (Bi2212) reveals that the spectral dip feature is directly linked to strong electronic coupling to a narrow boson spectrum, evidenced by a large peak in I'2F(I). The tunneling dip feature remains robust in the overdoped regime of Bi2212 with bulk Tc values of 56Â Ka62Â K. This is contrary to recent optical conductivity measurements of the self-energy that suggest the narrow boson spectrum disappears in overdoped Bi2212 and therefore cannot be essential for the pairing mechanism. The discrepancy is resolved by considering the way each technique probes the electron self-energy, in particular, the unique sensitivity of tunneling to the off-diagonal or pairing part of the self-energy.
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