Palladium-Catalysed Regio- and Stereoselective Arylative Substitution of Gamma,delta-Epoxy Esters and Amides by Sodium Tetraaryl Borates
| dc.contributor.author | Bilgi, Yasemin | |
| dc.contributor.author | Kuş, Melih | |
| dc.contributor.author | Artok, Levent | |
| dc.coverage.doi | 10.1039/d0ob01226b | |
| dc.date.accessioned | 2021-01-24T18:43:11Z | |
| dc.date.available | 2021-01-24T18:43:11Z | |
| dc.date.issued | 2020 | |
| dc.description.abstract | Palladium-catalysed reactions of gamma,delta-epoxy-alpha,beta-unsaturated esters and amides with NaBAr(4)reagents proceeded regio- and stereoselectively, producing allylic homoallyl alcohols with aryl-substituents in the allylic position for a wide range of substrates. AsPh(3)was found to be a competent ligand for the arylation reaction, whereas phosphine ligand/Lewis acidic organoboron combinations favoured the substitution reaction by oxygen nucleophiles (e.g.H2O, ROH). | en_US |
| dc.description.sponsorship | Scientific and Technological Research Council of TurkeyTurkiye Bilimsel ve Teknolojik Arastirma Kurumu (TUBITAK) [216Z094]; IZTECHIzmir Institute of Technology [2017YTE85] | en_US |
| dc.description.sponsorship | Dedicated in memory of Prof. D. Nuket ocal-Sungurolu. The financial support of the Scientific and Technological Research Council of Turkey (216Z094) and IZTECH (2017YTE85) is gratefully acknowledged. We thank Mr. S. Sakrak of Redoks Analytical Laboratory Equipments Ltd. Co., Dr. O. N. Aslan of Ataturk University, and Ms. T. Tunceli of Trakya University for HRMS analyses. | en_US |
| dc.identifier.doi | 10.1039/d0ob01226b | |
| dc.identifier.issn | 1477-0520 | |
| dc.identifier.issn | 1477-0539 | |
| dc.identifier.scopus | 2-s2.0-85089712350 | |
| dc.identifier.uri | https://doi.org/10.1039/d0ob01226b | |
| dc.identifier.uri | https://hdl.handle.net/11147/10444 | |
| dc.language.iso | en | en_US |
| dc.publisher | Royal Society of Chemistry | en_US |
| dc.relation.ispartof | Organic and Biomolecular Chemistry | en_US |
| dc.rights | info:eu-repo/semantics/closedAccess | en_US |
| dc.title | Palladium-Catalysed Regio- and Stereoselective Arylative Substitution of Gamma,delta-Epoxy Esters and Amides by Sodium Tetraaryl Borates | en_US |
| dc.type | Article | en_US |
| dspace.entity.type | Publication | |
| gdc.author.institutional | Bilgi, Yasemin | |
| gdc.author.institutional | Kuş, Melih | |
| gdc.author.institutional | Artok, Levent | |
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| gdc.description.department | İzmir Institute of Technology. Chemistry | en_US |
| gdc.description.endpage | 6383 | en_US |
| gdc.description.issue | 32 | en_US |
| gdc.description.publicationcategory | Makale - Uluslararası Hakemli Dergi - Kurum Öğretim Elemanı | en_US |
| gdc.description.scopusquality | Q3 | |
| gdc.description.startpage | 6378 | en_US |
| gdc.description.volume | 18 | en_US |
| gdc.description.wosquality | Q2 | |
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| gdc.identifier.pmid | 32756732 | |
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